Highly selective electroreduction of N2 and CO2 to urea over artificial frustrated Lewis pairs

Author:

Yuan Menglei12,Chen Junwu12,Xu Yong3,Liu Rongji4ORCID,Zhao Tongkun12,Zhang Jingxian12,Ren Zhongyu12,Liu Zhanjun5,Streb Carsten4ORCID,He Hongyan12ORCID,Yang Chao123ORCID,Zhang Suojiang12ORCID,Zhang Guangjin123ORCID

Affiliation:

1. CAS Key Laboratory of Green Process Engineering, Beijing Key Laboratory of Ionic Liquids Clean Process, State Key Laboratory of Multiphase Complex Systems, Institute of Process Engineering, Chinese Academy of Sciences, Beijing 100190, China

2. School of Chemical Engineering, Center of Materials Science and Optoeletronics Engineering, University of Chinese Academy of Sciences, Beijing 100190, China

3. Chemistry and Chemical Engineering Guangdong Laboratory, Shantou 515031, China

4. Institute of Inorganic Chemistry, Ulm University, Ulm 89081, Germany

5. State Key Laboratory of Coal Conversion, CAS Key Laboratory of Carbon Materials, Institute of Coal Chemistry, Chinese Academy of Sciences, Taiyuan 030001, China

Abstract

Precisely fabricated frustrated Lewis pairs in the Ni3(BO3)2 nanocrystal achieve integration of the active sites and effective electrocatalytic C–N bond coupling to synthesize urea.

Funder

National Natural Science Foundation of China

National Key Research and Development Program of China

Publisher

Royal Society of Chemistry (RSC)

Subject

Pollution,Nuclear Energy and Engineering,Renewable Energy, Sustainability and the Environment,Environmental Chemistry

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