Nitrogen adsorption on Nb2C6H4+ cations: the important role of benzyne (ortho-C6H4)-Reference-Cited by-同舟云学术

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Nitrogen adsorption on Nb₂C₆H₄⁺ cations: the important role of benzyne (ortho-C₆H₄)

Published:2024 Issue:5 Volume:26 Page:3912-3919
ISSN:1463-9076
Container-title:Physical Chemistry Chemical Physics
language:en
Short-container-title:Phys. Chem. Chem. Phys.

Author:

Zhang Feng-Xiang¹,Zhang Yi-Heng¹,Wang Ming¹,Ma Jia-Bi¹^ORCID

Affiliation:

1. Key Laboratory of Cluster Science of Ministry of Education, Beijing Key Laboratory of Photoelectronic/Electrophotonic Conversion Materials, School of Chemistry and Chemical Engineering, Beijing Institute of Technology, Beijing 102488, P. R. China

Abstract

Compared with the naked Nb2+, the Nb2C6H4+ cation, containing organic ligand ortho-C6H4, shows higher reactivity towards N2. This study indicates that organic ligands can be crucial to N2 adsorption and activation.

Funder

National Natural Science Foundation of China

National Key Research and Development Program of China

Beijing Municipal Natural Science Foundation

Publisher

Royal Society of Chemistry (RSC)

Link

http://pubs.rsc.org/en/content/articlepdf/2024/CP/D3CP05524H

Reference66 articles.

1. Dinitrogen Activation and Addition to Unsaturated C−E (E=C, N, O, S) Bonds Mediated by Transition Metal Complexes

2. Nitrogen fixation and transformation with main group elements

3. From Dinitrogen to N‐Containing Organic Compounds: Using Li₂CN₂ as a Synthon

4. Direct synthesis of cyanate anion from dinitrogen catalysed by molybdenum complexes bearing pincer-type ligand

5. Synthesis of pyrimidines from dinitrogen and carbon

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