A hot carrier perovskite solar cell with efficiency exceeding 27% enabled by ultrafast hot hole transfer with phthalocyanine derivatives

Author:

Gong Shaokuan1,Qu Geping23,Qiao Ying2,Wen Yifan1,Huang Yuling1,Cai Siyuan2,Zhang Letian2,Jiang Kui4,Liu Shang1,Lin Meng1ORCID,Beard Matthew C.5ORCID,Xu Zong-Xiang2,Chen Xihan1ORCID

Affiliation:

1. Shenzhen Key Laboratory of Intelligent Robotics and Flexible Manufacturing Systems, SUSTech Energy Institute for Carbon Neutrality, Department of Mechanical and Energy Engineering, Southern University of Science and Technology, Shenzhen, Guangdong 518055, China

2. Department of Chemistry, Southern University of Science and Technology, Shenzhen, Guangdong 518055, China

3. School of Chemistry and Chemical Engineering, Harbin Institute of Technology, Harbin, 150001, China

4. Department of Materials Science and Engineering, City University of Hong Kong, Kowloon, 999077, Hong Kong

5. National Renewable Energy Laboratory, Golden, CO, 80401, USA

Abstract

Illustration of hot hole transfer through interfacial S–Pb interactions, and a peak efficiency of 27.30% was achieved under 5.9 suns via ultrafast hot hole extraction.

Funder

Science, Technology and Innovation Commission of Shenzhen Municipality

Natural Science Foundation of Guangdong Province

Center for Hybrid Organic Inorganic Semiconductors for Energy

National Natural Science Foundation of China

Guangdong University of Science and Technology

Basic and Applied Basic Research Foundation of Guangdong Province

Basic Energy Sciences

National Renewable Energy Laboratory

Publisher

Royal Society of Chemistry (RSC)

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