Two-dimensional two-photon absorptions and third-order nonlinear optical properties of Ih fullerenes and fullerene onions

Author:

Zheng Xue-Lian12345,Yang Ling678910,Shang Bo12345ORCID,Wang Ming-Qian678910,Niu Yingli11121314,Li Wei-Qi159101416,Tian Wei Quan12345ORCID

Affiliation:

1. Chongqing Key Laboratory of Theoretical and Computational Chemistry

2. College of Chemistry and Chemical Engineering

3. Chongqing University

4. Huxi Campus

5. Chongqing 401331

6. MIIT Key Laboratory of Critical Materials Technology for New Energy Conversion and Storage

7. Institute of Theoretical and Simulational Chemistry

8. School of Chemistry and Chemical Engineering

9. Harbin Institute of Technology

10. Harbin 150001

11. School of Science

12. Beijing Jiaotong University

13. Beijing 100044

14. China

15. School of Physics

16. Collaborative Innovation Center of Extreme Optics

Abstract

The third order nonlinear optical properties of Ih symmetry fullerenes increase exponentially with fullerene size. The two-dimensional two-photon absorption spectra for C60 and C240 have strong self-phase modulation responses.

Funder

State Key Laboratory of Supramolecular Structure and Materials

National Natural Science Foundation of China

Graduate Scientific Research and Innovation Foundation of Chongqing

Beijing Jiaotong University

Publisher

Royal Society of Chemistry (RSC)

Subject

Physical and Theoretical Chemistry,General Physics and Astronomy

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