Synthesis of α-heterofunctionalized carbonyl compounds <i>via</i> Brønsted acid-catalyzed oxygenative coupling of ynamides-Reference-Cited by-同舟云学术

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Synthesis of α-heterofunctionalized carbonyl compounds via Brønsted acid-catalyzed oxygenative coupling of ynamides

Published:2024 Issue:6 Volume:11 Page:1790-1795
ISSN:2052-4129
Container-title:Organic Chemistry Frontiers
language:en
Short-container-title:Org. Chem. Front.

Author:

Um Tae-Woong¹²,Yeom Hyun-Suk²^ORCID,Shin Seunghoon¹^ORCID

Affiliation:

1. Department of Chemistry, Research Institute for Natural Sciences and Center for New Directions in Organic Synthesis (CNOS), Hanyang University, 222 Wangsimni-ro, Seongdong-gu, Seoul 04763, Korea

2. Eco-Friendly New Materials Research Center, Therapeutics & Biotechnology Division, Korea Research Institute of Chemical Technology (KRICT), 141 Gajeong-ro, Yuseong-gu, Daejeon, 34114, Korea

Abstract

Brønsted acid-catalyzed addition of pyridine-N-oxides to ynamides forms N-enoxypyridinium ions that are functionally equivalent to α-carbonyl cations.

Funder

National Research Foundation of Korea

Ministry of Science, ICT and Future Planning

Ministry of Trade, Industry and Energy

Publisher

Royal Society of Chemistry (RSC)

Link

http://pubs.rsc.org/en/content/articlepdf/2024/QO/D3QO02134C

Reference42 articles.

1. M.Uyanik , Catalytic oxidative α-functionalization of carbonyls , in Iodine Catalysis in Organic Synthesis , ed. K. Ishihara and K. Muniz , Wiley-VCH , 2022 , pp. 275–298

2. Transition Metal Catalyzed Enantioselective α-Heterofunctionalization of Carbonyl Compounds

3. Recent advances in the synthesis of α-amino ketones

4. Asymmetric hydroxylation of enolates with N-sulfonyloxaziridines

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