Improving the electrocatalytic N2 reduction activity of Pd nanoparticles through surface modification

Author:

Deng Guorong12345,Wang Ting67894ORCID,Alshehri Abdulmohsen Ali1011121314,Alzahrani Khalid Ahmad1011121314,Wang Yan52154,Ye Hejiang16174,Luo Yonglan67894ORCID,Sun Xuping1234ORCID

Affiliation:

1. Institute of Fundamental and Frontier Sciences

2. University of Electronic Science and Technology of China

3. Chengdu 610054

4. China

5. School of Materials and Energy

6. Chemical Synthesis and Pollution Control Key Laboratory of Sichuan Province

7. College of Chemistry and Chemical Engineering

8. China West Normal University

9. Nanchong 637002

10. Chemistry Department

11. Faculty of Science

12. King Abdulaziz University

13. Jeddah 21589

14. Saudi Arabia

15. Chengdu 611731

16. Hospital of Chengdu University of Traditional Chinese Medicine

17. Chengdu 610072

Abstract

Tannic acid (TA)-modified Pd nanoparticles (Pd-TA) are efficient for ambient electrocatalytic N2-to-NH3 fixation with an NH3 yield of 24.12 μg h−1 mgcat.−1 and a faradaic efficiency of 9.49%.

Funder

National Natural Science Foundation of China

Publisher

Royal Society of Chemistry (RSC)

Subject

General Materials Science,Renewable Energy, Sustainability and the Environment,General Chemistry

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