M–Ge–Si thermolytic molecular precursors and models for germanium-doped transition metal sites on silica

Author:

Dombrowski James P.12ORCID,Kalendra Vidmantas3,Ziegler Micah S.12ORCID,Lakshmi K. V.3ORCID,Bell Alexis T.24,Tilley T. Don12ORCID

Affiliation:

1. Department of Chemistry, University of California, Berkeley, Berkeley, CA, USA

2. Chemical Sciences Division, Lawrence Berkeley National Laboratory, 1 Cyclotron Road, Berkeley, CA, USA

3. Department of Chemistry and Chemical Biology and The Baruch ‘60 Center for Biochemical Solar Energy Research, Rensselaer Polytechnic Institute, Troy, NY 12180, USA

4. Department of Chemical and Biomolecular Engineering, University of California, Berkeley, 201 Gilman Hall, Berkeley, CA, USA

Abstract

The new siloxy-germoxy ligand HOGe[OSi(OtBu)3]3 generates Mn-, Fe-, and Cr-containing precursors suitable for thermolytic molecular precursor routes to quaternary oxides.

Funder

U.S. Department of Energy

National Institutes of Health

National Science Foundation

Publisher

Royal Society of Chemistry (RSC)

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