A general acetic acid vapour etching strategy to synthesize layered carbon nitride with carbon vacancies for efficient photoredox catalysis

Author:

Zhao Jianghong1,Mu Rihui1,Zhang Ya2,Yang Zhidong2,Zhang Hongxia2ORCID,Shi Hu23ORCID,Zhang Min2,Zheng Zhanfeng4ORCID,Yang Pengju24ORCID

Affiliation:

1. Engineering Research Center of Ministry of Education for Fine Chemicals, Shanxi University, Taiyuan 030006, China

2. School of Chemistry and Chemical Engineering, Shanxi University, Taiyuan 030006, China

3. Institute of Molecular Science, Shanxi University, Taiyuan 030006, China

4. State Key Laboratory of Coal Conversion, Institute of Coal Chemistry, Chinese Academy of Sciences, Taiyuan 030001, China

Abstract

A chemical etching strategy has been developed to prepare polymeric carbon nitride (PCN) nanosheets with carbon vacancies (CVs). The CVs can regulate the electronic properties of the Pt cocatalyst, thereby achieving superior hydrogen production.

Funder

National Natural Science Foundation of China

ShanXi Science and Technology Department

Natural Science Foundation of Shanxi Province

State Key Laboratory of Coal Conversion, Institute of Coal Chemistry, Chinese Academy of Sciences

Publisher

Royal Society of Chemistry (RSC)

Subject

General Materials Science,Renewable Energy, Sustainability and the Environment,General Chemistry

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