Gas-phase synthesis of [OU–X]+ (X = Cl, Br and I) from a UO22+ precursor using ion-molecule reactions and an [OUCH]+ intermediate-Reference-Cited by-同舟云学术

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Gas-phase synthesis of [OU–X]⁺ (X = Cl, Br and I) from a UO₂²⁺ precursor using ion-molecule reactions and an [OUCH]⁺ intermediate

Published:2024 Issue:12 Volume:53 Page:5478-5483
ISSN:1477-9226
Container-title:Dalton Transactions
language:en
Short-container-title:Dalton Trans.

Author:

Terhorst Justin¹^ORCID,Lenze Samuel¹,Metzler Luke¹^ORCID,Fry Allison N.¹,Ihabi Amina¹,Corcovilos Theodore A.²^ORCID,van Stipdonk Michael J.¹^ORCID

Affiliation:

1. Department of Chemistry and Biochemistry, Duquesne University, Pittsburgh, PA 15282, USA

2. Department of Physics, Duquesne University, Pittsburgh, PA 15282, USA

Abstract

Preparative tandem mass spectrometry can be used to dissociate the oxo ligands from UO22+; allowing generation of formally U(iv) oxy-halide ions [OU–X]+, (X = Cl, Br and I) via an [OUCH]+ intermediate.

Funder

Duquesne University

National Science Foundation

Publisher

Royal Society of Chemistry (RSC)

Link

http://pubs.rsc.org/en/content/articlepdf/2024/DT/D3DT02811A

Reference41 articles.

1. Elucidation of the collision induced dissociation pathways of water and alcohol coordinated complexes containing the uranyl cation

2. Gas-Phase Complexes Containing the Uranyl Ion and Acetone

3. Gas-Phase Uranyl−Nitrile Complex Ions

4. Production and collision-induced dissociation of gas-phase, water- and alcohol-coordinated uranyl complexes containing halide or perchlorate anions

5. Gas-Phase Coordination Complexes of Dipositive Plutonyl, PuO22+: Chemical Diversity Across the Actinyl Series

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