Tracking the solid-state incorporation of Sn into the framework of dealuminated zeolite beta, and consequences for catalyst design

Author:

Navar Ricardo1,Tarantino Giulia2ORCID,Beynon Owain T.1,Padovan Daniele1,Botti Luca2,Gibson Emma K.34ORCID,Wells Peter P.456ORCID,Owens Alun1,Kondrat Simon A.7ORCID,Logsdail Andrew J.1ORCID,Hammond Ceri2ORCID

Affiliation:

1. Cardiff Catalysis Institute, Cardiff University, Park Place, Cardiff, CF10 3AT, UK

2. Department of Chemical Engineering, Imperial College London, London, SW7 2AZ, UK

3. School of Chemistry, University of Glasgow, University Avenue, Glasgow, G12 8QQ, UK

4. UK Catalysis Hub, Research Complex at Harwell, Rutherford Appleton Laboratories, Harwell Science and Innovation Campus, Oxon, OX11 0FA, UK

5. School of Chemistry, University of Southampton, Southampton, SO17 1BJ, UK

6. Diamond Light Source Ltd, Didcot, Oxon, OX11 0DE, UK

7. Department of Chemistry, Loughborough University, Loughborough, LE11 3TU, UK

Abstract

In situ spectroscopy, kinetic studies and computational simulations are combined to study the synthesis of Sn-Beta by solid state incorporation, revealing which parameters influence successful preparation of the catalyst.

Funder

Engineering and Physical Sciences Research Council

Diamond Light Source

Consejo Nacional de Ciencia y Tecnología

Royal Society

Coleg Cymraeg Cenedlaethol

Publisher

Royal Society of Chemistry (RSC)

Subject

General Materials Science,Renewable Energy, Sustainability and the Environment,General Chemistry

Cited by 7 articles. 订阅此论文施引文献 订阅此论文施引文献,注册后可以免费订阅5篇论文的施引文献,订阅后可以查看论文全部施引文献

1. Computational study on 119Sn NMR for Sn-β Zeolites;Ninth International Symposium on Energy Science and Chemical Engineering (ISESCE 2024);2024-06-19

2. Deactivation and Reductive Regeneration of Sn-Beta for Liquid-Phase Biomass Conversion;ACS Catalysis;2024-05-10

3. Ordered and Disordered Metal Oxide for Biomass Conversion;The Materials Research Society Series;2023-10-26

4. Tracking Lattice Distortion Induced by Defects and Framework Tin in Beta Zeotypes;The Journal of Physical Chemistry C;2023-09-18

5. Computational Study of the Solid-State Incorporation of Sn(II) Acetate into Zeolite β;The Journal of Physical Chemistry C;2023-09-15

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