Light-driven oxidation of CH4 to C1 chemicals catalysed by an organometallic Ru complex with O2

Author:

Nakano Tatsuya1,Abe Tsukasa2ORCID,Matsumoto Takahiro134ORCID,Kimura Kento1,Nakamura Genta1,Hayami Shinya5ORCID,Shiota Yoshihito2ORCID,Yoshizawa Kazunari23ORCID,Ogo Seiji13ORCID

Affiliation:

1. Department of Chemistry and Biochemistry, Graduate School of Engineering, Kyushu University, 744 Moto-oka, Nishi-ku, Fukuoka 819-0395, Japan

2. Institute for Materials Chemistry and Engineering, Kyushu University, 744 Moto-oka, Nishi-ku, Fukuoka 819-0395, Japan

3. International Institute for Carbon-Neutral Energy Research (WPI-I2CNER), Kyushu University, 744 Moto-oka, Nishi-ku, Fukuoka, 819-0395, Japan

4. Precursory Research for Embryonic Science and Technology (PRESTO), Japan Science and Technology Agency (JST), Kawaguchi 332-0012, Japan

5. Graduate School of Science and Technology, Kumamoto University, 2-39-1 Kurokami, Chuo-ku, Kumamoto 860-8555, Japan

Abstract

We have achieved aerobic transformation of methane to C1 chemicals catalysed by a homogeneous organometallic catalyst with light energy input.

Funder

Precursory Research for Embryonic Science and Technology

Core Research for Evolutional Science and Technology

Publisher

Royal Society of Chemistry (RSC)

Subject

General Chemical Engineering,General Chemistry

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