Revisiting the photochemical synthesis of [FeFe]-hydrogenase mimics: reaction optimization, mechanistic study and electrochemical behaviour

Author:

Aguado Sergio12345ORCID,Casarrubios Luis12345ORCID,Ramírez de Arellano Carmen13678ORCID,Sierra Miguel A.12345ORCID

Affiliation:

1. Departamento de Química Orgánica

2. Facultad de Ciencias Químicas

3. Center for Innovation in Advanced Chemistry (ORFEO-CINQA)

4. Universidad Complutense

5. 28040-Madrid

6. Universidad de Valencia

7. 46100-Valencia

8. Spain

Abstract

The photochemistry of [(μ-S)2Fe2(CO)6] and alkenes or alkynes has been developed to a synthetically useful level. Computational data and electrochemistry of the photoadducts show interesting properties of these compounds.

Funder

Fundación Ramón Areces

Ministerio de Ciencia, Innovación y Universidades

Publisher

Royal Society of Chemistry (RSC)

Subject

General Chemical Engineering,General Chemistry

Reference64 articles.

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3. I.Dincer and C.Zamfirescu , Sustainable Hydrogen Production , Elsevier , 2016

4. Compendium of Hydrogen Energy Volume 4: Hydrogen Use, Safety and the Hydrogen Economy , ed. M. Ball , A. Basile and T. N. Veziroğlu , Elsevier , 2016

5. Comprehensive review and future perspectives on the photocatalytic hydrogen production

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