Selectivity switching resulting in the formation of benzene by surface carbonates on ceria in catalytic gas-phase oxidation of benzyl alcohol

Author:

Dai Yihu12345,Wu Xin-Ping67895,Tang Yu12345,Yang Yanhui10111213,Gong Xue-Qing67895,Fan Jie12345

Affiliation:

1. Key Lab of Applied Chemistry of Zhejiang Province

2. Department of Chemistry

3. Zhejiang University

4. Hangzhou 310027

5. People's Republic of China

6. Key Laboratory for Advanced Materials

7. Centre for Computational Chemistry and Research Institute of Industrial Catalysis

8. East China University of Science and Technology

9. Shanghai 200237

10. School of Chemical and Biomedical Engineering

11. Nanyang Technological University

12. Singapore 637459

13. Singapore

Abstract

The carbonate deposits on CeO2 cause the formation of benzene in gas-phase aerobic oxidation of benzyl alcohol via easy trapping of CO fragments.

Publisher

Royal Society of Chemistry (RSC)

Subject

Materials Chemistry,Metals and Alloys,Surfaces, Coatings and Films,General Chemistry,Ceramics and Composites,Electronic, Optical and Magnetic Materials,Catalysis

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