Selectivity switching resulting in the formation of benzene by surface carbonates on ceria in catalytic gas-phase oxidation of benzyl alcohol-Reference-Cited by-同舟云学术

Selectivity switching resulting in the formation of benzene by surface carbonates on ceria in catalytic gas-phase oxidation of benzyl alcohol

Published:2016 Issue:13 Volume:52 Page:2827-2830
ISSN:1359-7345
Container-title:Chemical Communications
language:en
Short-container-title:Chem. Commun.

Author:

Dai Yihu¹²³⁴⁵,Wu Xin-Ping⁶⁷⁸⁹⁵,Tang Yu¹²³⁴⁵,Yang Yanhui¹⁰¹¹¹²¹³,Gong Xue-Qing⁶⁷⁸⁹⁵,Fan Jie¹²³⁴⁵

Affiliation:

1. Key Lab of Applied Chemistry of Zhejiang Province

2. Department of Chemistry

3. Zhejiang University

4. Hangzhou 310027

5. People's Republic of China

6. Key Laboratory for Advanced Materials

7. Centre for Computational Chemistry and Research Institute of Industrial Catalysis

8. East China University of Science and Technology

9. Shanghai 200237

10. School of Chemical and Biomedical Engineering

11. Nanyang Technological University

12. Singapore 637459

13. Singapore

Abstract

The carbonate deposits on CeO₂ cause the formation of benzene in gas-phase aerobic oxidation of benzyl alcohol via easy trapping of CO fragments.

Publisher

Royal Society of Chemistry (RSC)

Subject

Materials Chemistry,Metals and Alloys,Surfaces, Coatings and Films,General Chemistry,Ceramics and Composites,Electronic, Optical and Magnetic Materials,Catalysis

Link

http://pubs.rsc.org/en/content/articlepdf/2016/CC/C5CC08904B

Reference29 articles.

1. Oxidation of Alcohols with Molecular Oxygen on Solid Catalysts

2. Solvent-Free Oxidation of Primary Alcohols to Aldehydes Using Au-Pd/TiO 2 Catalysts

3. Ordered Nanoporous Silica with Periodic 30−60 nm Pores as an Effective Support for Gold Nanoparticle Catalysts with Enhanced Lifetime

4. Hydroxyapatite-Supported Palladium Nanoclusters: A Highly Active Heterogeneous Catalyst for Selective Oxidation of Alcohols by Use of Molecular Oxygen

5. Origin of the High Activity of Mesoporous CeO2 Supported Monomeric VOx for Low-Temperature Gas-Phase Selective Oxidative Dehydrogenation of Benzyl Alcohol: Role As an Electronic “Hole”

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