Interplay of Purcell effect and extraction efficiency in CsPbBr3 quantum dots coupled to Mie resonators

Author:

He Ruihua1,Meunier Max23,Dong Zhaogang45ORCID,Cai Hongbing6,Gao Weibo367,Zuniga-Perez Jesus36ORCID,Liu Xiaogang1ORCID

Affiliation:

1. Department of Chemistry, National University of Singapore, Singapore 117543, Singapore

2. Université Côte d'Azur, CNRS, CRHEA, 06560 Valbonne, France

3. MajuLab, International Research Laboratory IRL 3654, CNRS, Université Côte d'Azur, Sorbonne Université, National University of Singapore, Nanyang Technological University, Singapore, Singapore

4. Institute of Materials Research and Engineering, A*STAR (Agency for Science, Technology and Research), 2 Fusionopolis Way, #08-03 Innovis, Singapore 138634, Singapore

5. Department of Materials Science and Engineering, National University of Singapore, 9 Engineering Drive 1, Singapore 117575, Singapore

6. Division of Physics and Applied Physics, School of Physical and Mathematical Sciences, Nanyang Technological University, 637371, Singapore

7. The Photonics Institute and Centre for Disruptive Photonic Technologies, Nanyang Technological University, 637371, Singapore

Abstract

Perovskites quantum dots coupled to Mie resonators display an 18-fold luminescence enhancement. Spatially- and time-resolved measurements, coupled to numerical simulations, confirm increased absorption, Purcell factor and extraction efficiency.

Funder

National Research Foundation

Institute of Materials Research and Engineering

Centre National de la Recherche Scientifique

Publisher

Royal Society of Chemistry (RSC)

Subject

General Materials Science

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