Hybridized local and charge transfer dendrimers with near-unity exciton utilization for enabling high-efficiency solution-processed hyperfluorescent OLEDs

Author:

Yin Yixiao1,Zeng Songkun1,Xiao Chen1,Fan Peng1,Shin Dong Jin2,Kim Ki Ju3,Nam Hyewon3,Ma Qian4,Ma Huili4ORCID,Zhu Weiguo1ORCID,Kim Taekyung35ORCID,Lee Jun Yeob26ORCID,Wang Yafei1ORCID

Affiliation:

1. Jiangsu Collaborative Innovation Center of Photovoltaic Science and Engineering, Jiangsu Engineering Laboratory of Light-Electricity-Heat Energy-Converting Materials and Applications, School of Materials Science & Engineering, Changzhou University, Changzhou 213164, China

2. School of Chemical Engineering, Sungkyunkwan University 2066, Seobu-ro, Jangan-gu, Gyeonggi, Suwon 14169, Korea

3. Department of Information Display, Hongik University, 04066, Seoul, Korea

4. Key Laboratory of Flexible Electronics (KLOFE) & Institute of Advanced Materials (IAM), Nanjing Tech University (NanjingTech), 30 South Puzhu Road, Nanjing 211816, China

5. Department of Materials Science and Engineering, Hongik University, Sejong, 30016, Korea

6. SKKU Institute of Energy Science and Technology, Sungkyunkwan University 2066, Seobu-ro, Jangan-gu, Suwon, Gyeonggi, 16419, Korea

Abstract

Two dendrimers, called D-TTT-H and D-TTT-tBu, were prepared, which exhibits both hot exciton process and TADF characteristic simultaneously in solid state. The solution processable OLED showed an EQEmax of 30.88% employing D-TTT-H as a sensitizer.

Funder

National Natural Science Foundation of China

Publisher

Royal Society of Chemistry (RSC)

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