Rational design of a carbon/potassium poly(heptazine imide) heterojunction for enhanced photocatalytic H2 and H2O2 evolution

Author:

Pelicano Christian Mark1ORCID,Li Jiaxin1,Cabrero-Antonino María2,Silva Ingrid F.1,Peng Lu1,Tarakina Nadezda V.1ORCID,Navalón Sergio2,García Hermenegildo2ORCID,Antonietti Markus1ORCID

Affiliation:

1. Department of Colloid Chemistry, Max Planck Institute of Colloids and Interfaces, Potsdam 14476, Germany

2. Departamento de Química, Instituto de Tecnología Química (CSIC-UPV), Universitat Politècnica de València, València 46022, Spain

Abstract

We construct a carbon/KPHI heterostructure for high-performance photocatalytic H2 and H2O2 evolution. The optimal 0.3Ad/KPHI hybrid showed an outstanding H2 evolution rate of 738 μmol h−1 gcat−1 and H2O2 production rate of 3.94 mmol h−1 gcat−1.

Funder

Alexander von Humboldt-Stiftung

Ministerio de Ciencia e Innovación

European Regional Development Fund

Publisher

Royal Society of Chemistry (RSC)

Subject

General Materials Science,Renewable Energy, Sustainability and the Environment,General Chemistry

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