Copper carbenes alkylate guanine chemoselectively through a substrate directed reaction-Reference-Cited by-同舟云学术

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Copper carbenes alkylate guanine chemoselectively through a substrate directed reaction

Published:2017 Issue:1 Volume:8 Page:499-506
ISSN:2041-6520
Container-title:Chemical Science
language:en
Short-container-title:Chem. Sci.

Author:

Geigle Stefanie N.¹²³⁴,Wyss Laura A.⁵⁶⁷⁴,Sturla Shana J.⁵⁶⁷⁴,Gillingham Dennis G.¹²³⁴

Affiliation:

1. Department of Chemistry

2. University of Basel

3. Basel

4. Switzerland

5. Department of Health Sciences and Technology

6. ETH Zurich

7. CH-8092 Zurich

Abstract

Cu(i) carbenes derived from α-diazocarbonyl compounds lead to selective alkylation of the O⁶position in guanine (O⁶-G) in mono- and oligonucleotides.

Funder

European Research Council

Eidgenössische Technische Hochschule Zürich

Swiss National Science Foundation

Publisher

Royal Society of Chemistry (RSC)

Subject

General Chemistry

Link

http://pubs.rsc.org/en/content/articlepdf/2017/SC/C6SC03502G

Reference69 articles.

1. M. A. M. M. P. Doyle and T.Ye, Modern Catalytic Methods for Organic Synthesis with Diazo Compounds, Wiley, New York, 1998

2. Modern Organic Synthesis with α-Diazocarbonyl Compounds

3. Catalytic X–H insertion reactions based on carbenoids

4. Asymmetric catalytic cyclopropanation reactions in water

5. Selective Tryptophan Modification with Rhodium Carbenoids in Aqueous Solution

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