Elucidation of the atomic-scale processes of dissociative adsorption and spillover of hydrogen on the single atom alloy catalyst Pd/Cu(111)

Author:

Osada Wataru1,Tanaka Shunsuke1,Mukai Kozo1,Kawamura Mitsuaki1ORCID,Choi YoungHyun1,Ozaki Fumihiko1,Ozaki Taisuke1,Yoshinobu Jun1ORCID

Affiliation:

1. The Institute for Solid State Physics, The University of Tokyo, 5-1-5 Kashiwanoha, Kashiwa, Chiba 277-8581, Japan

Abstract

The dissociative adsorption and spillover processes of hydrogen on the Pd deposited Cu(111) surface were investigated using IRAS, TPD, HR-XPS, and DFT calculations, which have elucidated the atomic-scale perspective of hydrogen on Pd/Cu(111).

Funder

Japan Society for the Promotion of Science

Japan Science and Technology Agency

Ministry of Education, Culture, Sports, Science and Technology

Publisher

Royal Society of Chemistry (RSC)

Subject

Physical and Theoretical Chemistry,General Physics and Astronomy

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