Mechanistic study of NHC-catalyzed oxidative N <i>vs</i>. O chemoselective acylation of aldehydes with alkanolamines-Reference-Cited by-同舟云学术

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Mechanistic study of NHC-catalyzed oxidative N vs. O chemoselective acylation of aldehydes with alkanolamines

Published:2024 Issue:24 Volume:48 Page:11159-11172
ISSN:1144-0546
Container-title:New Journal of Chemistry
language:en
Short-container-title:New J. Chem.

Author:

Sang Yuan¹,Joseph Ojo¹,Yuan Hai-Yan¹,Zhang Jing-Ping¹^ORCID

Affiliation:

1. Jilin Province Key Laboratory of Organic Functional Molecular Design & Synthesis, Advanced Energy Materials Research Center, Faculty of Chemistry, Northeast Normal University, Renmin Street 5268#, Changchun 130024, P. R. China

Abstract

We studied the mechanism of NHC-catalyzed oxidative amidation of aryl aldehydes and amines, the sources of chemoselectivity, and the role of additives through DFT calculations.

Funder

National Natural Science Foundation of China

Fundamental Research Funds for the Central Universities

Publisher

Royal Society of Chemistry (RSC)

Link

http://pubs.rsc.org/en/content/articlepdf/2024/NJ/D4NJ00189C

Reference69 articles.

1. Alternative and Uncommon Acylating Agents – An Alive and Kicking Methodology

2. Stability-increasing effects of anthocyanin glycosyl acylation

3. Reductive Arylation of Amides via a Nickel‐Catalyzed Suzuki–Miyaura‐Coupling and Transfer‐Hydrogenation Cascade

4. Synthesis and Pharmacological Characterization of a Series of Geometrically Constrained 5-HT2A/2C Receptor Ligands

5. Kinetic Resolution and Deracemization of Racemic Amines Using a Reductive Aminase

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