Singlet oxygen is not the main source of electrolyte degradation in lithium–oxygen batteries

Author:

Zor Ceren1ORCID,Jones Kieran D.23ORCID,Rees Gregory J.12ORCID,Yang Sixie1,Pateman Alexander1,Gao Xiangwen1,Johnson Lee R.234ORCID,Bruce Peter G.124ORCID

Affiliation:

1. Department of Materials, University of Oxford, Oxford, UK

2. The Faraday Institution, Quad One, Harwell Science and Innovation Campus, Didcot OX11 0RA, UK

3. Nottingham Applied Materials and Interfaces Group, School of Chemistry, University of Nottingham, Nottingham, UK

4. Department of Chemistry, University of Oxford, Oxford, UK

Abstract

The lithium–oxygen field has focused on singlet oxygen’s role in cell degradation. This study shows no significant reaction between singlet oxygen and the electrolyte or carbon cathode, confirming it is not the major degradation source.

Funder

EPSRC Centre for Doctoral Training in Additive Manufacturing

Henry Royce Institute

Publisher

Royal Society of Chemistry (RSC)

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