Thiazoloisoindigo-based ambipolar polymers for excellent balanced hole and electron mobility

Author:

Li Bowen1,Zou Xiangyu1,Xiong Miao2,Li Qiyi2,Kang Xu3,Mu Youbing1,Wang Jieyu2,Pei Jian2ORCID,Yang Chunming4,Lan Zhenggang3ORCID,Wan Xiaobo1ORCID

Affiliation:

1. School of Optoelectronic Materials & Technology, Key Laboratory of Opto-electronic Chemical Materials and Devices, Ministry of Education, Jianghan University, Wuhan, 430056, P. R. China

2. Beijing National Laboratory for Molecular Sciences, the Key Laboratory of Bioorganic Chemistry and Molecular Engineering of Ministry of Education, College of Chemistry and Molecular Engineering, Peking University, Beijing 100871, P. R. China

3. SCNU Environmental Research Institute, Guangdong Provincial Key Laboratory of Chemical Pollution and Environmental Safety & MOE Key Laboratory of Environmental Theoretical Chemistry, School of Environment, South China Normal University, Guangzhou 510006, P. R. China

4. Shanghai Synchrotron Radiation Facility, Shanghai Advanced Research Institute, Chinese Academy of Sciences, Shanghai, 201204, P. R. China

Abstract

The copolymerization of thiophene-flanked thiazoisoindigo (TzII) and thiophene-flanked dipyrrolopyrrolidone (DPP) leads to an ambipolar polymer with high and balanced charge carrier mobility (highest μe: 7.63 and highest μh: 6.11 cm2 V−1 s−1, respectively).

Funder

National Natural Science Foundation of China

Jianghan University

Publisher

Royal Society of Chemistry (RSC)

Subject

Materials Chemistry,General Materials Science

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