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Electric fields drive bond homolysis

Published:2023 Issue:7 Volume:14 Page:1769-1774
ISSN:2041-6520
Container-title:Chemical Science
language:en
Short-container-title:Chem. Sci.

Author:

Zhang Boyuan¹^ORCID,Schaack Cedric²^ORCID,Prindle Claudia R.²,Vo Ethan A.²,Aziz Miriam²^ORCID,Steigerwald Michael L.²,Berkelbach Timothy C.²³,Nuckolls Colin²^ORCID,Venkataraman Latha¹²^ORCID

Affiliation:

1. Department of Applied Physics and Applied Mathematics, Columbia University, New York 10027, New York, US

2. Department of Chemistry, Columbia University, New York 10027, New York, USA

3. Center for Computational Quantum Physics, Flatiron Institute, New York, New York, 10010, USA

Abstract

We demonstrate that electric fields can homolytically cleave a peroxide bond in different solvents with a rate that is proportional to the solvent dielectric constant.

Funder

National Science Foundation

National Defense Science and Engineering Graduate

Publisher

Royal Society of Chemistry (RSC)

Subject

General Chemistry

Link

http://pubs.rsc.org/en/content/articlepdf/2023/SC/D2SC06411A

Reference47 articles.

1. Electrostatic Basis for Enzyme Catalysis

2. Remarkably Selective Iridium Catalysts for the Elaboration of Aromatic C-H Bonds

3. Low-pressure hydrogenolysis of glycerol to propylene glycol

4. Dehydration of glycerol to acetol via catalytic reactive distillation

5. Enantiomerically Enriched Allylic Alcohols and Allylic Amines via C–C Bond-Forming Hydrogenation: Asymmetric Carbonyl and Imine Vinylation

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