Effect of hydrophilicity-imparting substituents on exciton delocalization in squaraine dye aggregates covalently templated to DNA Holliday junctions

Author:

Pascual Gissela1ORCID,Roy Simon K.1ORCID,Barcenas German1,Wilson Christopher K.1,Cervantes-Salguero Keitel1ORCID,Obukhova Olena M.2,Krivoshey Alexander I.2,Terpetschnig Ewald A.3,Tatarets Anatoliy L.2,Li Lan1,Yurke Bernard14,Knowlton William B.14,Mass Olga A.1ORCID,Pensack Ryan D.1ORCID,Lee Jeunghoon15ORCID

Affiliation:

1. Micron School of Materials Science & Engineering, Boise State University, Boise, Idaho 83725, USA

2. State Scientific Institution “Institute for Single Crystals” of the National Academy of Sciences of Ukraine, Kharkiv 61072, Ukraine

3. SETA BioMedicals, LLC, Urbana, Illinois 61801, USA

4. Department of Electrical & Computer Engineering, Boise State University, Boise, Idaho 83725, USA

5. Department of Chemistry and Biochemistry, Boise State University, Boise, Idaho 83725, USA

Abstract

Molecular aggregates exhibit collective sharing of electronic excitation energy known as exciton delocalization, that can be leveraged in applications such as quantum computing, optical information processing, and light harvesting.

Funder

U.S. Department of Energy

Publisher

Royal Society of Chemistry (RSC)

Subject

General Materials Science

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