Rh(iii)-catalyzed regioselective intermolecular N-methylene Csp3–H bond carbenoid insertion
Author:
Affiliation:
1. School of Chemistry and Chemical Engineering
2. South China University of Technology
3. Guangzhou
4. P. R. China
5. School of Materials Science & Engineering
6. PCFM Lab
7. Sun Yat-sen University
Abstract
A Rh(iii)-catalyzed regioselective intermolecular carbenoid insertion into the N-methylene Csp3–H bond has been achieved via an outer-sphere pathway.
Funder
National Natural Science Foundation of China
Guangdong Natural Science Foundation
Publisher
Royal Society of Chemistry (RSC)
Subject
General Chemistry
Link
http://pubs.rsc.org/en/content/articlepdf/2018/SC/C7SC03802J
Reference40 articles.
1. Catalytic Enantioselective C−H Activation by Means of Metal−Carbenoid-Induced C−H Insertion
2. The Combined C–H Functionalization/Cope Rearrangement: Discovery and Applications in Organic Synthesis
3. Catalytic Enantioselective Synthesis of β2-Amino Acids This work was supported by the National Science Foundation (CHE 0092490) and the National Institutes of Health (GM57425).
4. Double C−H Activation Strategy for the Asymmetric Synthesis of C2-Symmetric Anilines
5. Enantioselective synthesis of β-amino esters and its application to the synthesis of the enantiomers of the antidepressant Venlafaxine
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