Continuous-flow reactor with superior production rate and stability for CO2 reduction using semiconductor photocatalysts

Author:

Jung Hyunju12ORCID,Kim Chansol3,Yoo Hae-Wook4ORCID,You Jei5,Kim Jin Seog5,Jamal Aqil6,Gereige Issam6,Ager Joel W.27ORCID,Jung Hee-Tae18ORCID

Affiliation:

1. Department of Chemical and Biomolecular Engineering, Korea Advanced Institute of Science and Technology (KAIST), 291 Daehak-ro, Yuseong-gu, Daejeon 34141, South Korea

2. Chemical Sciences Division, Lawrence Berkeley National Laboratory, 1 Cyclotron Road, Berkeley, California 94720, USA

3. Clean Energy Research Center, Korea Institute of Science and Technology (KIST), Hwarang-ro 14-gil 5, Seongbuk-gu, Seoul 02792, South Korea

4. The First R&D Institute, Agency for Defense Development, Yuseong-gu, Daejeon 305-600, South Korea

5. Gas Isotope Metrology Team, Korea Research Institute of Standards and Science, Daejeon 34113, South Korea

6. Saudi Aramco, Research and Development Center, Dhahran, 31311, Saudi Arabia

7. Department of Materials Science and Engineering, University of California Berkeley, California 94720, USA

8. Korea Advanced Institute of Science and Technology (KAIST) Institute for Nanocentury, Daejeon 34141, South Korea

Abstract

A new semiconductor-based photocatalytic reactor design with optimized pressure and flow rates on both sides of an intermediately placed catalyst enhances mass transport, accelerates CO desorption and prevents photocatalyst deactivation.

Funder

National Research Foundation of Korea

U.S. Department of Energy

Office of Science

Basic Energy Sciences

Saudi Aramco

Publisher

Royal Society of Chemistry (RSC)

Subject

Pollution,Nuclear Energy and Engineering,Renewable Energy, Sustainability and the Environment,Environmental Chemistry

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