Interfacial Co–O–Cu bonds prompt electrochemical nitrate reduction to ammonia in neutral electrolyte-Reference-Cited by-同舟云学术

Interfacial Co–O–Cu bonds prompt electrochemical nitrate reduction to ammonia in neutral electrolyte

Published:2024 Issue:20 Volume:60 Page:2756-2759
ISSN:1359-7345
Container-title:Chemical Communications
language:en
Short-container-title:Chem. Commun.

Author:

Yao Kai¹,Fang Zhaobin¹,Yan Weijie¹,Wang Yawu¹,Song Zhenyong¹,Wang Wenhai¹,Wang Jieyue¹,Wei Xianwen¹,Tan Yiwei²,Wu Dehong³,Wu Konglin¹^ORCID,Jiang Binbin⁴^ORCID

Affiliation:

1. Institute of Clean Energy and Advanced Nanocatalysis (iClean), School of Chemistry and Chemical Engineering, Anhui University of Technology, Maanshan 243032, China

2. State Key Laboratory of Materials-Oriented Chemical Engineering, Nanjing University of Technology, Nanjing 211816, China

3. Emergency Management Bureau of Jiangan County, Yibin 644200, China

4. School of Chemistry and Chemical Engineering, Anqing Normal University, Anqing 246001, China

Abstract

The Co–O–Cu interfacial bonds in Co2–Cu(OH)2 sufficiently expose active sites and improve the reaction kinetics. The optimal Co2–Cu(OH)2 provides an amazing electrocatalytic performance for the NO3RR.

Funder

National Natural Science Foundation of China

Anhui Provincial Department of Education

Publisher

Royal Society of Chemistry (RSC)

Link

http://pubs.rsc.org/en/content/articlepdf/2024/CC/D3CC05801H

Reference41 articles.

1. Non-aqueous gas diffusion electrodes for rapid ammonia synthesis from nitrogen and water-splitting-derived hydrogen

2. Anchor single atom in h-BN assist NO synthesis NH3: a computational view

3. A rigorous electrochemical ammonia synthesis protocol with quantitative isotope measurements

4. Breaking scaling relations to achieve low-temperature ammonia synthesis through LiH-mediated nitrogen transfer and hydrogenation

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