Selective hydrogen–deuterium exchange in graphitic carbon nitrides: probing the active sites for photocatalytic water splitting by solid-state NMR-Reference-Cited by-同舟云学术

Selective hydrogen–deuterium exchange in graphitic carbon nitrides: probing the active sites for photocatalytic water splitting by solid-state NMR

Published:2021 Issue:7 Volume:9 Page:3985-3994
ISSN:2050-7488
Container-title:Journal of Materials Chemistry A
language:en
Short-container-title:J. Mater. Chem. A

Author:

Wang Ruidi¹²³⁴⁵,Xu Bei-Bei¹²³⁴⁵,Wang Jiachen¹²³⁴⁵,Wang Xue Lu¹²³⁴⁵,Yao Ye-Feng¹²³⁴⁵^ORCID

Affiliation:

1. Physics Department & Shanghai Key Laboratory of Magnetic Resonance

2. School of Physics and Materials Science

3. East China Normal University

4. Shanghai 200062

5. P. R. China

Abstract

By selective deuteration, the exchangeable and unexchangeable protons of the H-containing groups of g-C₃N₄ were differentiated, providing a way to distinguish the hydrophilic and relatively non-hydrophilic H-containing groups of g-C₃N₄.

Funder

Ministry of Science and Technology of the People's Republic of China

National Natural Science Foundation of China

Publisher

Royal Society of Chemistry (RSC)

Subject

General Materials Science,Renewable Energy, Sustainability and the Environment,General Chemistry

Link

http://pubs.rsc.org/en/content/articlepdf/2021/TA/D0TA10148F

Reference37 articles.

1. Recent development in graphitic carbon nitride based photocatalysis for hydrogen generation

2. Solar Synthesis: Prospects in Visible Light Photocatalysis

3. Rapid high-temperature treatment on graphitic carbon nitride for excellent photocatalytic H2-evolution performance

4. Solar Hydrogen Generation by a CdS-Au-TiO2 Sandwich Nanorod Array Enhanced with Au Nanoparticle as Electron Relay and Plasmonic Photosensitizer

5. Local spatial charge separation and proton activation induced by surface hydroxylation promoting photocatalytic hydrogen evolution of polymeric carbon nitride

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