Decoupling Li+ conductivity and mechanical stability in a thermally reversible concentrated sulfone-based gel electrolyte for lithium metal batteries

Author:

Jiang Xueao1,Chen Jiayin1,Zeng Junfeng1,Liu Weijian1,Wu Xuansheng1,Lv Yang1,Liu Fangyan2,Zhang Ce3,Li Zhiyong4ORCID,Wang Xiwen1ORCID,Zhang Shiguo1ORCID

Affiliation:

1. State Key Laboratory of Advanced Design and Manufacturing Technology for Vehicle, College of Materials Science and Engineering, Hunan University, Changsha 410082, P. R. China

2. Department of Physics, City University of Hong Kong, Hong Kong 999077, Hong Kong

3. Nanophotonics and Optoelectronics Research Center, Qian Xuesen Laboratory of Space Technology, China Academy of Space Technology, Beijing 100094, China

4. School of Chemistry and Chemical Engineering, Henan Normal University, Xinxiang, Henan 453007, P. R. China

Abstract

This work presents a mechanically strong and highly Li+-conductive gel electrolyte featuring thermally induced electrode wetting and healing, which holds great promise in solid-state lithium-metal batteries and other flexible and wearable devices.

Funder

Natural Science Foundation of Hunan Province

National Natural Science Foundation of China

State Key Laboratory of Advanced Design and Manufacturing for Vehicle Body

Henan Normal University

Publisher

Royal Society of Chemistry (RSC)

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