Monitoring the active sites for the hydrogen evolution reaction at model carbon surfaces-Reference-Cited by-同舟云学术

Monitoring the active sites for the hydrogen evolution reaction at model carbon surfaces

Published:2021 Issue:16 Volume:23 Page:10051-10058
ISSN:1463-9076
Container-title:Physical Chemistry Chemical Physics
language:en
Short-container-title:Phys. Chem. Chem. Phys.

Author:

Kluge Regina M.¹²³⁴⁵,Haid Richard W.¹²³⁴⁵,Stephens Ifan E. L.⁶⁷⁸⁹¹⁰,Calle-Vallejo Federico¹¹¹²¹³¹⁴^ORCID,Bandarenka Aliaksandr S.¹²³⁴⁵^ORCID

Affiliation:

1. Physics of Energy Conversion and Storage

2. Physik-Department

3. Technische Universität München

4. 85748 Garching

5. Germany

6. Department of Materials

7. Imperial College London

8. Royal School of Mines

9. London

10. UK

11. Departament de Ciència de Materials i Química Física & Institut de Química Teòrica i Computacional (IQTCUB)

12. Universitat de Barcelona

13. 08028 Barcelona

14. Spain

Abstract

We determine the active sites for the H₂ evolution on carbon in acid with atomic resolution using scanning tunneling microscopy and density functional theory. While terraces remain inactive, the most active sites are found at steps and defects.

Funder

Deutsche Forschungsgemeinschaft

Horizon 2020

Ministerio de Ciencia, Innovación y Universidades

Generalitat de Catalunya

Publisher

Royal Society of Chemistry (RSC)

Subject

Physical and Theoretical Chemistry,General Physics and Astronomy

Link

http://pubs.rsc.org/en/content/articlepdf/2021/CP/D1CP00434D

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