Thermodynamics of the formation of surface PtO2 stripes on Pt(111) in the absence of subsurface oxygen-Reference-Cited by-同舟云学术

Thermodynamics of the formation of surface PtO2 stripes on Pt(111) in the absence of subsurface oxygen

Published:2020 Issue:19 Volume:22 Page:10634-10640
ISSN:1463-9076
Container-title:Physical Chemistry Chemical Physics
language:en
Short-container-title:Phys. Chem. Chem. Phys.

Author:

Hanselman Selwyn¹²³⁴,McCrum Ian T.¹²³⁴,Rost Marcel J.⁵²⁶⁴,Koper Marc T. M.¹²³⁴^ORCID

Affiliation:

1. Leiden Institute of Chemistry

2. Leiden University

3. 2300 RA Leiden

4. The Netherlands

5. Huygens-Kamerlingh Onnes Laboratory

6. 2333 CA Leiden

Abstract

This paper examines the thermodynamics of PtO₂ stripes formed as intermediates of Pt(111) surface oxidation as a function of the degree of dilation parallel to the stripes, using density functional theory and atomistic thermodynamics.

Funder

Nederlandse Organisatie voor Wetenschappelijk Onderzoek

H2020 Marie Skłodowska-Curie Actions

Publisher

Royal Society of Chemistry (RSC)

Subject

Physical and Theoretical Chemistry,General Physics and Astronomy

Link

http://pubs.rsc.org/en/content/articlepdf/2020/CP/C9CP05107D

Reference33 articles.

1. CO Oxidation on Pt(110): Scanning Tunneling Microscopy Inside a High-Pressure Flow Reactor

2. Structure and Reactivity of Surface Oxides on Pt(110) during Catalytic CO Oxidation

3. The mechanism of the catalytic action of platinum in the reactions 2Co + O2= 2Co2 and 2H2+ O2= 2H2O

4. Initial stages of Pt(111) electrooxidation: dynamic and structural studies by surface X-ray diffraction

5. Influence of Electrolyte Composition and pH on Platinum Electrochemical and/or Chemical Dissolution in Aqueous Acidic Media

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