ZIF-8 pyrolized N-doped carbon-supported iron catalysts for enhanced CO2 hydrogenation activity to valuable hydrocarbons

Author:

Deng Chao1,Wang Xu1ORCID,Chen Xixi1,Gao Ruxing2,Zhang Leiyu1,Zhang Chundong1ORCID,Jun Ki-Won34,Kim Seok Ki5,Wan Hui1,Guan Guofeng16ORCID

Affiliation:

1. State Key Laboratory of Materials-Oriented Chemical Engineering, College of Chemical Engineering, Nanjing Tech University, Nanjing, 211816, P. R. China

2. School of Energy Science and Engineering, Nanjing Tech University, Nanjing, 211816, P. R. China

3. C1 Gas Separation and Conversion Research Group, Carbon Resources Institute, Korea Research Institute of Chemical Technology (KRICT), Yuseong, Daejeon 34114, Republic of Korea

4. Advanced Materials and Chemical Engineering, Korea University of Science and Technology (UST), Yuseong, Daejeon, 34113, Republic of Korea

5. Department of Chemical Engineering, Ajou University, Suwon 16499, Republic of Korea

6. Xitai Lake Industrial College, Nanjing Tech University, Changzhou 213149, PR China

Abstract

The N atom in the nitrogen-doped carbon materials can promote the adsorption and conversion of CO2. In addition, as a bridge between N and Fe, the degree of graphitization of carbon supports significantly affects the electron transfer process.

Funder

Ministry of Science and ICT, South Korea

Natural Science Foundation of Jiangsu Province

Publisher

Royal Society of Chemistry (RSC)

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