Coordinatively unsaturated nickel–nitrogen sites towards selective and high-rate CO2electroreduction

Author:

Yan Chengcheng12345,Li Haobo12345,Ye Yifan12345,Wu Haihua12345,Cai Fan12345,Si Rui67589ORCID,Xiao Jianping12345,Miao Shu12345,Xie Songhai10111289,Yang Fan12345ORCID,Li Yanshuo131114159,Wang Guoxiong12345ORCID,Bao Xinhe12345ORCID

Affiliation:

1. State Key Laboratory of Catalysis

2. CAS Center for Excellence in Nanoscience

3. Dalian National Laboratory for Clean Energy

4. Dalian Institute of Chemical Physics

5. Chinese Academy of Sciences

6. Shanghai Synchrotron Radiation Facility

7. Shanghai Institute of Applied Physics

8. Shanghai

9. China

10. Shanghai Key Laboratory of Molecular Catalysis and Innovative Materials

11. Department of Chemistry

12. Fudan University

13. School of Material Science and Chemical Engineering

14. Ningbo University

15. Ningbo

Abstract

Coordinatively unsaturated Ni–N active sites facilitate CO2electroreduction and inhibit the competitive hydrogen evolution reaction, demonstrating selective and high-rate CO2electroreduction.

Funder

Ministry of Science and Technology of the People's Republic of China

National Natural Science Foundation of China

Chinese Academy of Sciences

Dalian Institute of Chemical Physics

Publisher

Royal Society of Chemistry (RSC)

Subject

Pollution,Nuclear Energy and Engineering,Renewable Energy, Sustainability and the Environment,Environmental Chemistry

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