Efficient electrohydrogenation of N2 to NH3 by oxidized carbon nanotubes under ambient conditions

Author:

Zhao Jinxiu1234,Wang Bo56784,Zhou Qiang1234,Wang Huanbo910114,Li Xianghong121314154,Chen Hongyu123416ORCID,Wei Qin121314154ORCID,Wu Dan121314154ORCID,Luo Yonglan16617184ORCID,You Jinmao56784,Gong Feng (Frank)1920214ORCID,Sun Xuping1234ORCID

Affiliation:

1. Institute of Fundamental and Frontier Sciences

2. University of Electronic Science and Technology of China

3. Chengdu 610054

4. China

5. Key Laboratory of Life-Organic Analysis of Shandong Province

6. College of Chemistry and Chemical Engineering

7. Qufu Normal University

8. Qufu 273165

9. School of Environment and Resource

10. Southwest University of Science and Technology

11. Mianyang 621010

12. Key Laboratory of Chemical Sensing & Analysis in Universities of Shandong

13. School of Chemistry and Chemical Engineering

14. University of Jinan

15. Jinan 250022

16. Chemical Synthesis and Pollution Control Key Laboratory of Sichuan Province

17. China West Normal University

18. Nanchong 637002

19. School of Energy and Environment

20. Southeast University

21. Nanjing 211189

Abstract

As a metal-free electrocatalyst for the N2 reduction reaction, oxidized carbon nanotubes attain NH3 yield of 32.33 mg h−1 mgcat.−1 and faradaic efficiency of 12.50%.

Funder

National Natural Science Foundation of China

Publisher

Royal Society of Chemistry (RSC)

Subject

Materials Chemistry,Metals and Alloys,Surfaces, Coatings and Films,General Chemistry,Ceramics and Composites,Electronic, Optical and Magnetic Materials,Catalysis

Reference49 articles.

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