Reversal of methanation-oriented to RWGS-oriented Ni/SiO<sub>2</sub> catalysts by the exsolution of Ni<sup>2+</sup> confined in silicalite-1-Reference-Cited by-同舟云学术

Reversal of methanation-oriented to RWGS-oriented Ni/SiO₂ catalysts by the exsolution of Ni²⁺ confined in silicalite-1

Published:2023 Issue:19 Volume:25 Page:7582-7597
ISSN:1463-9262
Container-title:Green Chemistry
language:en
Short-container-title:Green Chem.

Author:

Chen Chia-Hung¹,Chen Hong-Kai¹,Huang Wei-Hsiang²,Chen Chi-Liang²^ORCID,Choojun Kittisak³⁴,Sooknoi Tawan³⁴^ORCID,Tian Hong-Kang¹⁵^ORCID,Lin Yu-Chuan¹^ORCID

Affiliation:

1. Department of Chemical Engineering, National Cheng Kung University, Tainan 70101, Taiwan

2. National Synchrotron Radiation Research Center, Hsinchu 30076, Taiwan

3. Department of Chemistry, School of Science, King Mongkut's Institute of Technology Ladkrabang, Chalongkrung Road, Ladkrabang, Bangkok 10520, Thailand

4. Catalytic Chemistry Research Unit, School of Science, King Mongkut's Institute of Technology Ladkrabang, Chalongkrung Road, Ladkrabang, Bangkok 10520, Thailand

5. Hierarchical Green-Energy Materials (Hi-GEM) Research Center, National Cheng Kung University, Tainan 70101, Taiwan

Abstract

Ni/SiO2-based catalysts derived from the reduction of silicalite-1-encapsulated, ligand-protected Ni2+ was found to be effective in the selective hydrogenation of CO2 to CO via the reverse water-gas shift (RWGS).

Funder

National Cheng Kung University

National Science and Technology Council

Publisher

Royal Society of Chemistry (RSC)

Subject

Pollution,Environmental Chemistry

Link

http://pubs.rsc.org/en/content/articlepdf/2023/GC/D3GC02399K

Reference75 articles.

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2. A thermodynamic analysis of methanation reactions of carbon oxides for the production of synthetic natural gas

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