Rhodium(ii)-catalyzed C–H aminations using N-mesyloxycarbamates: reaction pathway and by-product formation-Reference-Cited by-同舟云学术

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Rhodium(ii)-catalyzed C–H aminations using N-mesyloxycarbamates: reaction pathway and by-product formation

Published:2019 Issue:3 Volume:10 Page:718-729
ISSN:2041-6520
Container-title:Chemical Science
language:en
Short-container-title:Chem. Sci.

Author:

Azek Emna¹²³,Khalifa Maroua¹²³,Bartholoméüs Johan¹²³,Ernzerhof Matthias¹²³,Lebel Hélène¹²³^ORCID

Affiliation:

1. Département de Chimie

2. Université de Montréal

3. Canada H3C3J7

Abstract

DFT study to elucidate the mechanism of Rh-catalyzed C–H aminations with N-mesyloxycarbamates and the pathway by which by-products formed.

Funder

Canada Research Chairs

Natural Sciences and Engineering Research Council of Canada

Canada Foundation for Innovation

Ministère de l'Économie, de la Science et de l'Innovation - Québec

Fonds de Recherche du Québec - Nature et Technologies

Université de Montréal

Publisher

Royal Society of Chemistry (RSC)

Subject

General Chemistry

Link

http://pubs.rsc.org/en/content/articlepdf/2019/SC/C8SC03153C

Reference91 articles.

1. Transition Metal-Catalyzed C–H Amination: Scope, Mechanism, and Applications

2. Transition metal-catalyzed iodine(iii)-mediated nitrene transfer reactions: efficient tools for challenging syntheses

3. Organic azides: “energetic reagents” for the intermolecular amination of C–H bonds

4. Intramolecular C(sp3)–H amination

5. Asymmetric Nitrene Transfer Reactions: Sulfimidation, Aziridination and C-H Amination Using Azide Compounds as Nitrene Precursors

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