First principles study on Li metallic phase nucleation at grain boundaries in a lithium lanthanum titanium oxide (LLTO) solid electrolyte-Reference-Cited by-同舟云学术

First principles study on Li metallic phase nucleation at grain boundaries in a lithium lanthanum titanium oxide (LLTO) solid electrolyte

Published:2023 Issue:6 Volume:11 Page:2889-2898
ISSN:2050-7488
Container-title:Journal of Materials Chemistry A
language:en
Short-container-title:J. Mater. Chem. A

Author:

Kim Hyungjun¹^ORCID,Conlin Patrick²^ORCID,Bergschneider Matthew²^ORCID,Chung Hayoung³,Kim Sung Youb³^ORCID,Cha Suk Won¹^ORCID,Cho Maenghyo¹^ORCID,Cho Kyeongjae²^ORCID

Affiliation:

1. Department of Mechanical Engineering, Seoul National University, Gwanak-ro, Gwanak-gu, Seoul 08826, Republic of Korea

2. Department of Materials Science and Engineering, The University of Texas at Dallas, Richardson, Texas, 75080, USA

3. Department of Mechanical Engineering, Ulsan National Institute of Science and Technology (UNIST), Ulsan 44919, Republic of Korea

Abstract

Among various intergranular microstructures, pore spaces in SEs play a critical role in Li-metal nucleation in SEs. To realize Li-metal nuclei-free inside the SE, removing pore spaces is essential and a commonly applicable design strategy to all SEs.

Funder

National Research Foundation of Korea

Korea Institute of Science and Technology Information

University of Texas at Austin

Publisher

Royal Society of Chemistry (RSC)

Subject

General Materials Science,Renewable Energy, Sustainability and the Environment,General Chemistry

Link

http://pubs.rsc.org/en/content/articlepdf/2023/TA/D2TA07950J

Reference52 articles.

1. Pathways for practical high-energy long-cycling lithium metal batteries

2. The rechargeable revolution: A better battery

3. Lithium Metal Anodes: Toward an Improved Understanding of Coupled Morphological, Electrochemical, and Mechanical Behavior

4. Challenges in Lithium Metal Anodes for Solid-State Batteries

Cited by 3 articles. 订阅此论文施引文献订阅此论文施引文献，注册后可以免费订阅5篇论文的施引文献，订阅后可以查看论文全部施引文献

1. Machine Learning for High-Throughput Configuration Sampling of Li−La−Ti−O Disordered Solid-State Electrolyte;The Journal of Physical Chemistry C;2024-08-19

2. Initiation of dendritic failure of LLZTO via sub-surface lithium deposition;Energy & Environmental Science;2024

3. Going against the Grain: Atomistic Modeling of Grain Boundaries in Solid Electrolytes for Solid-State Batteries;ACS Materials Au;2023-10-05