Identification of C2–C5 products from CO2 hydrogenation over PdZn/TiO2–ZSM-5 hybrid catalysts-Reference-Cited by-同舟云学术

Identification of C2–C5 products from CO2 hydrogenation over PdZn/TiO2–ZSM-5 hybrid catalysts

Published:2021 Issue: Volume:230 Page:52-67
ISSN:1359-6640
Container-title:Faraday Discussions
language:en
Short-container-title:Faraday Discuss.

Author:

Ruiz Esquius Jonathan¹²³⁴⁵^ORCID,Bahruji Hasliza⁶⁷⁸⁹^ORCID,Bowker Michael¹²³⁴⁵^ORCID,Hutchings Graham J.¹²³⁴⁵^ORCID

Affiliation:

1. School of Chemistry

2. Cardiff Catalysis Institute

3. Cardiff University

4. Cardiff CF10 3AT

5. UK

6. Centre of Advanced Material and Energy Science

7. University Brunei Darussalam

8. Gadong BE 1410

9. Brunei Darussalam

Abstract

PdZn/TiO₂ combined with ZSM-5 zeolites allowed for consecutive CO₂ hydrogenation to CH₃OH, CH₃OH dehydration to DME, and MTH/DMTH in a one-pass single bed reactor. PdZn alloys, although stable at high temperature, hydrogenate olefins, limiting MTH/DMTH chain growth.

Funder

Engineering and Physical Sciences Research Council

Publisher

Royal Society of Chemistry (RSC)

Subject

Physical and Theoretical Chemistry

Link

http://pubs.rsc.org/en/content/articlepdf/2021/FD/D0FD00135J

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