Cooperative N–H bond activation by amido-Ge(ii) cations-Reference-Cited by-同舟云学术

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Cooperative N–H bond activation by amido-Ge(ii) cations

Published:2020 Issue:27 Volume:49 Page:9495-9504
ISSN:1477-9226
Container-title:Dalton Transactions
language:en
Short-container-title:Dalton Trans.

Author:

Zhou Xueer¹²³⁴⁵,Vasko Petra¹²³⁴⁵^ORCID,Hicks Jamie¹²³⁴⁵^ORCID,Fuentes M. Ángeles¹²³⁴⁵^ORCID,Heilmann Andreas¹²³⁴⁵,Kolychev Eugene L.¹²³⁴⁵^ORCID,Aldridge Simon¹²³⁴⁵^ORCID

Affiliation:

1. Department of Chemistry

2. University of Oxford

3. Inorganic Chemistry Laboratory

4. Oxford

5. UK

Abstract

Germylium-ylidene cations, [R(L)Ge]⁺, featuring amido substituents at R and NHC or phosphine donors at L have been synthesized and structurally characterized. The Lewis acidic germanium cation and proximal amide function allow for facile cleavage of N–H bonds in 1,2 fashion.

Funder

Academy of Finland

Leverhulme Trust

Engineering and Physical Sciences Research Council

FP7 People: Marie-Curie Actions

Publisher

Royal Society of Chemistry (RSC)

Subject

Inorganic Chemistry

Link

http://pubs.rsc.org/en/content/articlepdf/2020/DT/D0DT01960G

Reference87 articles.

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3. 1,1,2,2,2,2,3,3,3,3-Decacarbonyl-1-(η-cyclohexa-1,3-diene)-triangulo-triosmium: a novel intermediate in synthetic osmium cluster chemistry

4. Reactions of water and ammonia with bis(pentamethylcyclopentadienyl) complexes of zirconium and hafnium

5. Nitrogen-hydrogen activation. 1. Oxidative addition of ammonia to iridium(I). Isolation, structural characterization and reactivity of amidoiridium hydrides

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3. Chemistry with weakly coordinating aluminates [Al(ORF)4]− and borates [B(ORF)4]−: From fundamentals to application;Comprehensive Inorganic Chemistry III;2023

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