Unexpected intramolecular N-arylcyano-β-diketiminate cyclization in new aminoquinoline derivative complexes of aluminium for CO2 fixation into cyclic carbonates-Reference-Cited by-同舟云学术

Unexpected intramolecular N-arylcyano-β-diketiminate cyclization in new aminoquinoline derivative complexes of aluminium for CO2 fixation into cyclic carbonates

Published:2019 Issue:30 Volume:43 Page:12059-12068
ISSN:1144-0546
Container-title:New Journal of Chemistry
language:en
Short-container-title:New J. Chem.

Author:

Moreno da Costa David¹²³⁴⁵,Borja Luis¹²³⁴⁵,Verdugo Camilo¹²³⁴⁵,Martinez Javier¹²³⁴⁵^ORCID,Quintero Celso¹²³⁴⁵,Jaque Pablo⁶⁷⁸⁴⁵^ORCID,Trofymchuk Oleksandra S.⁹¹⁰¹¹⁵,Daniliuc Constantin G.¹²¹³¹⁴¹⁵^ORCID,Cabrera Alan R.¹²³⁴⁵^ORCID,Rojas Rene S.¹²³⁴⁵^ORCID

Affiliation:

1. Departamento de Química Inorgánica

2. Facultad de Química y de Farmacia

3. Pontificia Universidad Católica de Chile

4. Santiago

5. Chile

6. Departamento de Química Orgánica y Fisicoquímica

7. Facultad de Ciencias Químicas y Farmacéuticas

8. Universidad de Chile

9. Núcleo Científico Multidisciplinario-DI

10. University of Talca

11. Talca

12. Organisch-Chemisches Institut

13. Universität Münster

14. Münster

15. Germany

Abstract

exo-Dig intramolecular cyclization of β-diketiminates allowed to obtain 4-amino-3-iminoquinolines ligands through a novel pathway. Al(III) complexes bearing these ligands where active towards the synthesis of cyclic carbonates from epoxides and CO₂.

Funder

Fondo Nacional de Desarrollo Científico y Tecnológico

Comisión Nacional de Investigación Científica y Tecnológica

Publisher

Royal Society of Chemistry (RSC)

Subject

Materials Chemistry,General Chemistry,Catalysis

Link

http://pubs.rsc.org/en/content/articlepdf/2019/NJ/C9NJ02499A

Reference61 articles.

1. The (β‐Diketiminato)bismuth(III) Complex [LBiCl(μ‐Cl)] 2 {L = HC[(CMe)(NAr)] 2 , Ar = 2,6‐ i Pr 2 C 6 H 3 } and Its Derivatives: The Presence of Versatile Ligand Ligation Modes

2. The chemistry of univalent metal β-diketiminates

3. Highly Electron‐Rich β‐Diketiminato Systems: Synthesis and Coordination Chemistry of Amino‐Functionalized “ N ‐nacnac” Ligands

4. Novel lithium 3-sila- and 3-germa-β-diketiminates†‡

5. Syntheses, characterizations and thermal analyses of four novel unsymmetrical β-diketiminates

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