A synthetic biological quantum optical system

Author:

Lishchuk Anna1234ORCID,Kodali Goutham5678ORCID,Mancini Joshua A.5678ORCID,Broadbent Matthew1234,Darroch Brice1234,Mass Olga A.91108,Nabok Alexei1112134ORCID,Dutton P. Leslie5678,Hunter C. Neil142154ORCID,Törmä Päivi1617181920ORCID,Leggett Graham J.1234ORCID

Affiliation:

1. Department of Chemistry

2. University of Sheffield

3. Sheffield S3 7HF

4. UK

5. The Johnson Research Foundation and Department of Biochemistry and Biophysics

6. University of Pennsylvania

7. Philadelphia

8. USA

9. N. Carolina State University

10. Raleigh

11. Materials and Engineering Research Institute

12. Sheffield Hallam University

13. Sheffield S1 1WB

14. Department of Molecular Biology and Biotechnology

15. Sheffield S10 2TN

16. COMP Centre of Excellence

17. Department of Applied Physics

18. Aalto University

19. School of Science

20. 00076 Aalto

Abstract

Strong coupling between plasmon modes and chlorins in synthetic light-harvesting maquette proteins yields hybrid light–matter states (plexcitons) whose energies are controlled by design of protein structure, enabling the creation of new states not seen under weak coupling.

Funder

Engineering and Physical Sciences Research Council

Basic Energy Sciences

Academy of Finland

Biotechnology and Biological Sciences Research Council

H2020 European Research Council

Publisher

Royal Society of Chemistry (RSC)

Subject

General Materials Science

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