Band gap modulation in zirconium-based metal–organic frameworks by defect engineering

Author:

Taddei Marco1234ORCID,Schukraft Giulia M.56784,Warwick Michael E. A.1234ORCID,Tiana Davide9101112ORCID,McPherson Matthew J.1234ORCID,Jones Daniel R.1234,Petit Camille56784ORCID

Affiliation:

1. Energy Safety Research Institute

2. Swansea University

3. Swansea

4. UK

5. Barrer Centre

6. Department of Chemical Engineering

7. Imperial College London

8. SW7 2AZ London

9. School of Chemistry

10. University College Cork

11. Cork T12 K8AF

12. Ireland

Abstract

A simple defect engineering approach to systematically tune the band gap of the prototypical zirconium-based metal–organic framework UiO-66 is reported. Defect engineered materials display enhanced photocatalytic activity.

Funder

European Regional Development Fund

Engineering and Physical Sciences Research Council

H2020 Marie Skłodowska-Curie Actions

University of Edinburgh

Publisher

Royal Society of Chemistry (RSC)

Subject

General Materials Science,Renewable Energy, Sustainability and the Environment,General Chemistry

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