Shallow conductance decay along the heme array of a single tetraheme protein wire

Author:

Garg Kavita1,Futera Zdenek2ORCID,Wu Xiaojing3,Jeong Yongchan1,Chiu Rachel4ORCID,Pisharam Varun Chittari1ORCID,Ha Tracy Q.1,Aragonès Albert C.5ORCID,van Wonderen Jessica H.4ORCID,Butt Julea N.4ORCID,Blumberger Jochen3,Díez-Pérez Ismael1ORCID

Affiliation:

1. Department of Chemistry, Faculty of Natural, Mathematical & Engineering Sciences, King's College London, Britannia House, 7 Trinity Street, London SE1 1DB, UK

2. Faculty of Science, University of South Bohemia, Branisovska 1760, 370 05 Ceske Budejovice, Czech Republic

3. Department of Physics and Astronomy, Thomas Young Centre, University College London, Gower Street, London WC1E 6BT, UK

4. School of Chemistry, School of Biological Sciences, University of East Anglia, Norwich Research Park, Norwich, NR4 7TJ, UK

5. Departament de Ciència de Materials i Química Física, Universitat de Barcelona, Institut de Química Teòrica i Computacional (IQTC), Marti i Franquès 1, 08028 Barcelona, Spain

Abstract

Small tetraheme cytochromes (STCs) support efficient electron tunnelling suggesting tunnelling-assisted long-range charge transport in large multiheme structures.

Funder

Engineering and Physical Sciences Research Council

Biotechnology and Biological Sciences Research Council

Grantová Agentura České Republiky

European Research Council

Ministerio de Ciencia e Innovación

Max-Planck-Gesellschaft

Publisher

Royal Society of Chemistry (RSC)

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