Realizing horizontal magnesium platelet deposition and suppressed surface passivation for high-performance magnesium metal batteries

Author:

Yang Gaoliang1ORCID,Li Yuanjian1,Wang Jianbiao1ORCID,Lum Yanwei1,Lim Carina Yi Jing1ORCID,Ng Man-Fai2ORCID,Zhang Chang3,Chang Zhi4,Zhang Zhonghan5,Handoko Albertus D.1ORCID,Ghosh Tanmay1ORCID,Li Shuzhou5ORCID,Sofer Zdenek6ORCID,Liu Wei3ORCID,Yao Yan78,Seh Zhi Wei1ORCID

Affiliation:

1. Institute of Materials Research and Engineering (IMRE), Agency for Science, Technology and Research (A*STAR), 2 Fusionopolis Way, Innovis #08-03, Singapore 138634, Republic of Singapore

2. Institute of High Performance Computing (IHPC), Agency for Science, Technology and Research (A*STAR), 1 Fusionopolis Way, #16-16 Connexis, Singapore 138632, Republic of Singapore

3. School of Physical Science and Technology, ShanghaiTech University, Shanghai 201210, China

4. Department of Materials Physics and Chemistry, School of Materials Science & Engineering, Central South University, Changsha, 410083, Hunan, China

5. School of Materials Science and Engineering, Nanyang Technological University, 50 Nanyang Ave, Singapore 639798, Republic of Singapore

6. Department of Inorganic Chemistry, University of Chemistry and Technology Prague, Technická 5, 166 28 Prague 6, Czech Republic

7. Department of Electrical and Computer Engineering, University of Houston, Houston, TX 77204, USA

8. Texas Center for Superconductivity at the University of Houston (TcSUH), University of Houston, Houston, TX 77204, USA

Abstract

1-chloropropane is introduced into conventional electrolytes to manipulate the kinetics and surface chemistry of Mg anodes, achieving suppressed passivation and planar Mg deposition with enhanced (002) orientations for efficient Mg metal batteries.

Funder

Grantová Agentura České Republiky

Publisher

Royal Society of Chemistry (RSC)

Subject

Pollution,Nuclear Energy and Engineering,Renewable Energy, Sustainability and the Environment,Environmental Chemistry

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