Real-time regeneration of a working zeolite monitored <i>via operando</i> X-ray diffraction and crystallographic imaging: how coke flees the MFI framework-Reference-Cited by-同舟云学术

Real-time regeneration of a working zeolite monitored via operando X-ray diffraction and crystallographic imaging: how coke flees the MFI framework

Published:2022 Issue:44 Volume:51 Page:16845-16851
ISSN:1477-9226
Container-title:Dalton Transactions
language:en
Short-container-title:Dalton Trans.

Author:

Kalantzopoulos Georgios N.¹,Rojo Gama Daniel¹,Pappas Dimitrios K.¹^ORCID,Dovgaliuk Iurii²³,Olsbye Unni¹^ORCID,Beato Pablo⁴^ORCID,Lundegaard Lars F.⁴,Wragg David S.¹^ORCID,Svelle Stian¹^ORCID

Affiliation:

1. Center for Materials Science and Nanotechnology (SMN), Department of Chemistry, University of Oslo, P.O. Box 1033, Blindern, N-0315 Oslo, Norway

2. Swiss-Norwegian Beamline at the European Synchrotron Facility, 71 avenue des Martyrs, F-38000, Grenoble, France

3. Institut des Matériaux Poreux de Paris, Département de Chimie, ENS - UMR 8004 CNRS-ENS-ESPCI, 24 rue Lhomond, 75005 Paris, France

4. Haldor Topsøe A/S, Haldor Topsøes Allé 1, 2800 Kgs, Lyngby, Denmark

Abstract

X-ray diffraction is used to investigate regeneration of an H-ZSM-5 zeolite catalyst used in the conversion of methanol to hydrocarbons.

Funder

Norges Forskningsråd

Publisher

Royal Society of Chemistry (RSC)

Subject

Inorganic Chemistry

Link

http://pubs.rsc.org/en/content/articlepdf/2022/DT/D2DT02845J

Reference50 articles.

1. The conversion of methanol and other O-compounds to hydrocarbons over zeolite catalysts

2. Conversion of Methanol to Hydrocarbons: How Zeolite Cavity and Pore Size Controls Product Selectivity

3. Methanol-to-hydrocarbons: catalytic materials and their behavior

4. Conversion of Methanol to Alkenes over Medium- and Large-Pore Acidic Zeolites: Steric Manipulation of the Reaction Intermediates Governs the Ethene/Propene Product Selectivity

5. Conversion of methanol to hydrocarbons over zeolite H-ZSM-5: On the origin of the olefinic species

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