Discerning molecular-level CO2 adsorption behavior in amine-modified sorbents within a controlled CO2/H2O environment towards direct air capture

Author:

Song Ah-Young12ORCID,Young John3ORCID,Wang Jieyu1,Fricke Sophia N.1ORCID,Piscina Katia3,Giovine Raynald4ORCID,Garcia Susana3,van der Spek Mijndert3ORCID,Reimer Jeffrey A.12ORCID

Affiliation:

1. Department of Chemical and Biomolecular Engineering, University of California, Berkeley, CA 94720, USA

2. Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, CA 94720, USA

3. Research Centre for Carbon Solutions, Heriot-Watt University, Edinburgh, EH14 4AS, UK

4. College of Chemistry Pines Magnetic Resonance Center - Core Facility, University of California, Berkeley, CA 94720, USA

Abstract

CO2 adsorption is influenced by its concentration and H2O presence. While concentration governs chemisorbed species formation, H2O significantly impacts CO2 adsorption capacity, especially under dilute conditions mimicking direct air capture (DAC).

Funder

National Science Foundation

Grantham Foundation for the Protection of the Environment

Publisher

Royal Society of Chemistry (RSC)

Reference61 articles.

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3. R.Bergman and A.Anatoly , The Case for Carbon Dioxide Removal: From Science to Justice , Carbon Dioxide Removal Primer, CDR Primer , 2021

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