Do grain boundaries dominate non-radiative recombination in CH3NH3PbI3 perovskite thin films?

Author:

Yang Mengjin1234,Zeng Yining5234,Li Zhen1234ORCID,Kim Dong Hoe1234,Jiang Chun-Sheng6234,van de Lagemaat Jao1234ORCID,Zhu Kai1234

Affiliation:

1. Chemistry and Nanoscience Center

2. National Renewable Energy Laboratory

3. Golden

4. USA

5. Biosciences Center

6. Material Science Center

Abstract

We examine grain boundaries (GBs) with respect to non-GB regions in high-quality perovskite films using fluorescence-lifetime imaging. We show that recombination happens in the non-GB regions and that GBs are not transparent to photogenerated carriers.

Funder

Solar Energy Technologies Program

Basic Energy Sciences

Publisher

Royal Society of Chemistry (RSC)

Subject

Physical and Theoretical Chemistry,General Physics and Astronomy

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