Manipulation of the crystalline phase diagram of hydrogen through nanoscale confinement effects in porous carbons-Reference-Cited by-同舟云学术

Manipulation of the crystalline phase diagram of hydrogen through nanoscale confinement effects in porous carbons

Published:2022 Issue:19 Volume:14 Page:7250-7261
ISSN:2040-3364
Container-title:Nanoscale
language:en
Short-container-title:Nanoscale

Author:

Terry Lui R.¹^ORCID,Rols Stephane²^ORCID,Tian Mi³^ORCID,da Silva Ivan⁴^ORCID,Bending Simon J.⁵^ORCID,Ting Valeska P.¹^ORCID

Affiliation:

1. Department of Mechanical Engineering, University of Bristol, BS8 1TR UK

2. Institut Laue-Langevin (ILL), Grenoble, France

3. College of Engineering, Mathematics and Physical Sciences, University of Exeter, EX4 4QF, UK

4. ISIS Neutron Source, Rutherford Appleton Laboratory, Harwell Oxford, Didcot OX11 0QX, UK

5. Department of Physics, University of Bath, Bath BA2 7AY, UK

Abstract

Confinement of H2 in subnanometre pores of microporous carbon stabilizes the lowest energy crystal confirmation at higher temperatures. Change in H2 phase behaviour shown to be caused by severe loss of rotational freedom and energy upon confinement.

Funder

Engineering and Physical Sciences Research Council

Science and Technology Facilities Council

Engineer Research and Development Center

Publisher

Royal Society of Chemistry (RSC)

Subject

General Materials Science

Link

http://pubs.rsc.org/en/content/articlepdf/2022/NR/D2NR00587E

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