Single and dual metal atom catalysts for enhanced singlet oxygen generation and oxygen reduction reaction

Author:

Tamtaji Mohsen1,Cai Songhhua2,Wu Wenting3ORCID,Liu Tongchao4,Li Zhimin2,Chang Hsun-Yun5ORCID,Galligan Patrick Ryan1,Iida Shin-ichi5ORCID,Li Xiangrong1,Rehman Faisal16ORCID,Amine Khalil4ORCID,Goddard William A.6ORCID,Luo Zhengtang1ORCID

Affiliation:

1. Department of Chemical and Biological Engineering, Guangdong-Hong Kong-Macao Joint Laboratory for Intelligent Micro-Nano Optoelectronic Technology, William Mong Institute of Nano Science and Technology, Hong Kong Branch of Chinese National Engineering Research Center for Tissue Restoration and Reconstruction, The Hong Kong University of Science and Technology, Clear Water Bay, Kowloon, Hong Kong, 999077, P. R. China

2. Department of Applied Physics, The Hong Kong Polytechnic University, Hunghom, Kowloon 999077, Hong Kong

3. State Key Laboratory of Heavy Oil Processing, College of Chemistry and Chemical Engineering, Institute of New Energy, China University of Petroleum (East China), Qingdao 266580, P. R. China

4. Chemical Sciences and Engineering Division, Argonne National Laboratory, 9700 Cass Ave, Lemont, IL 60439, USA

5. ULVAC-PHI, Inc., Analytical Laboratory, 2500 Hagisono, Chigasaki, Kanagawa 253-8522, Japan

6. Materials and Process Simulation Center (MSC), MC 139-74, California Institute of Technology, Pasadena, CA, 91125, USA

Abstract

We demonstrate rational design of graphene-supported single and dual metal atom catalysts (SACs and DACs) for photocatalytic applications, such as singlet oxygen (1O2) sensitization and H2O2 production.

Funder

Research Grants Council, University Grants Committee

Basic Energy Sciences

Innovation and Technology Commission

Guangdong Science and Technology Department

National Science Foundation

Publisher

Royal Society of Chemistry (RSC)

Subject

General Materials Science,Renewable Energy, Sustainability and the Environment,General Chemistry

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