Methyl substitution for noncentrosymmetric stacking: a promising organic single crystal for highly efficient terahertz-wave generation

Author:

Shi Jingkai12345,He Yixin67895,Liang Fei1011125ORCID,Zhang Xinyuan12345ORCID,Xu Degang67895,Yao Jiyong1314151617ORCID,Zhang Guochun1314151617,Hu Zhanggui12345,Yao Jianquan67895,Wu Yicheng12345

Affiliation:

1. Tianjin Key Laboratory of Functional Crystal Materials

2. Institute of Functional Crystals

3. Tianjin University of Technology

4. Tianjin 300384

5. China

6. The Institute of Laser & Optoelectronics

7. College of Precision Instruments and Opto-electronics Engineering

8. Tianjin University

9. Tianjin 300072

10. State Key Laboratory of Crystal Materials and Institute of Crystal Materials

11. Shandong University

12. Jinan 250100

13. Key Laboratory of Functional Crystals and Laser Technology

14. Beijing Center for Crystal Research and Development

15. Technical Institute of Physics and Chemistry

16. Chinese Academy of Sciences

17. Beijing 100190

Abstract

Acentric indolium-based OHI-T (C26H27NO4S) was obtained through rational design, and highly efficient terahertz-wave generation was realized using an OHI-T single crystal.

Funder

National Natural Science Foundation of China

Publisher

Royal Society of Chemistry (RSC)

Subject

Materials Chemistry,General Chemistry

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