Copper-catalyzed asymmetric 1,6-conjugate addition of <i>in situ</i> generated <i>para</i>-quinone methides with β-ketoesters-Reference-Cited by-同舟云学术

Copper-catalyzed asymmetric 1,6-conjugate addition of in situ generated para-quinone methides with β-ketoesters

Published:2022 Issue:46 Volume:58 Page:6653-6656
ISSN:1359-7345
Container-title:Chemical Communications
language:en
Short-container-title:Chem. Commun.

Author:

Wang Yi-Feng¹^ORCID,Wang Chao-Jie¹,Feng Qing-Zhou¹,Zhai Jing-Jing¹^ORCID,Qi Suo-Suo¹,Zhong Ai-Guo²,Chu Ming-Ming³^ORCID,Xu Dan-Qian¹^ORCID

Affiliation:

1. State Key Laboratory Breeding Base of Green Chemistry-Synthesis Technology, Key Laboratory of Green Pesticides and Cleaner Production Technology of Zhejiang Province, Department of Green Chemistry and Technology, Zhejiang University of Technology, Hangzhou 310014, P. R. China

2. Taizhou College of Pharmaceutical and Chemical Engineering, 318000, Taizhou, Zhejiang, P. R. China

3. College of Biological, Chemical Sciences and Engineering, Jiaxing University, Jiaxing 314001, P. R. China

Abstract

The first example of transition metal catalyzed asymmetric transformations of the in situ generated p-QMs has been developed, avoiding using pre-synthesized p-QMs requiring bulky 2,6-substitutions.

Funder

National Key Research and Development Program of China

Publisher

Royal Society of Chemistry (RSC)

Subject

Materials Chemistry,Metals and Alloys,Surfaces, Coatings and Films,General Chemistry,Ceramics and Composites,Electronic, Optical and Magnetic Materials,Catalysis

Link

http://pubs.rsc.org/en/content/articlepdf/2022/CC/D2CC00146B

Reference35 articles.

1. Total Synthesis of Kendomycin: A Macro−C−Glycosidation Approach

2. Syntheses and Absolute Stereochemistries of UPA0043 and UPA0044, Cytotoxic Antibiotics Having a p-Quinone-methide Structure

3. Evolution of a Total Synthesis of (−)-Kendomycin Exploiting a Petasis−Ferrier Rearrangement/Ring-Closing Olefin Metathesis Strategy

4. Asymmetric Catalytic 1,6-Conjugate Addition/Aromatization ofpara-Quinone Methides: Enantioselective Introduction of Functionalized Diarylmethine Stereogenic Centers

5. A New Organocatalytic Concept for Asymmetric α-Alkylation of Aldehydes

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